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I have to say that the best ones are the ones where the villainess is actually villainous. And I don't mean that dumbass "by revealing the cruel truth about these abusive pieces of shit, I'm actually being evil because I'm doing it for my own sake".
If all the people around you are actually cruel and unkind to you, the new cute girl especially likes to bully you for no reason and you've never done anything wrong, then sorry, you're not a villainess and don't belong in this anthology, because you're obviously a heroine.
I don't mind if the "heroine" is actually evil or whatever, but you can't just have this villainess be the nicest dish rag under the sun, with beauty befitting a heroine and act like she's actually in any way villainous. Sorry, no, being studious is actually a classic heroine trait, you're not suddenly evil because you study to be a good queen.